Disentangling the contribution of the transboundary out-flow from the Asian continent to Tokyo, Japan
- 주제(키워드) Contributions to aerosols in Tokyo , Long range transport , Size-segregated elements , Size-segregated ion components , Urban aerosol , Urban site
- 관리정보기술 faculty
- 등재 SCIE, SCOPUS
- 발행기관 Elsevier Ltd
- 발행년도 2021
- URI http://www.dcollection.net/handler/ewha/000000182096
- 본문언어 영어
- Published As http://dx.doi.org/10.1016/j.envpol.2021.117280
- 저작권 이화여자대학교 논문은 저작권에 의해 보호받습니다.
초록/요약
We assessed the contribution of transboundary air pollutants (TAPs) transported from China to Tokyo using the Pb(0.5<Dp < 1)/Cu(2.5<Dp < 10) index. We conducted intensive observations over four seasons during 2014–2015 and analyzed ionic components and thirteen elements in size-segregated aerosols collected at the top of a 30-m-high tower in a hilly forested area of the Field Museum Tamakyuryo (FM Tama), in a western suburb of Tokyo. In order to evaluate if the Pb(0.5<Dp < 1)/Cu(2.5<Dp < 10) ratio can be applied in Tokyo as the megacity, the annual average concentration of Pb at Cape Hedo, Kumamoto city, on the west side of Japan, was higher than that of Pb at Tokyo, on the east side; this result indicates that TAPs affect western Japan more than eastern Japan. We inferred the main source of Cu to be braking abrasion from cars at local scale on the basis of its enrichment factor and size distribution. From the Pb(0.5<Dp < 1)/Cu(2.5<Dp < 10) ratio and sulfate concentration, we inferred that the highest contribution of TAPs to the total mass concentration in Tokyo occurred in spring, when TAPs accounted for 55%, 72%, and 53% of the total mass concentration in the 0.1 < Dp < 0.5, 0.5 < Dp < 1, and 1 < Dp < 2.5 fractions, respectively. These results can contribute to assessment of TAPs in Tokyo. © 2021 Elsevier Ltd
more